Hi ddee,
To disable “Connect to Outlook” function in document library, I would suggest you to hide the ribbon button for the library.
To do this, you can create a SharePoint project using VS, and use CAML function to do this, here is an example:
Walkthrough: Removing a Button from the Server Ribbon:
http://msdn.microsoft.com/en-us/library/ff408060.aspx
Thanks,
Qiao Wei
TechNet Community Support
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