The Sysprep folder is a read only folder in System 32. I was getting the same File not found error.
Use the LeaveDebugMode to allow System.Diagnostics.Process component of out the state that
lets you interact with OS processes that run in special mode. The below code worked for me:
System.Security.SecureString pwd = new System.Security.SecureString();
pwd.AppendChar('x');
pwd.AppendChar('x');
pwd.AppendChar('x');
pwd.AppendChar('x');
pwd.AppendChar('x');
pwd.AppendChar('x');
pwd.AppendChar('x');
Process.LeaveDebugMode();
Process.Start("C:\\windows\\system32\\sysprep\\sysprep.exe", "<enter your user ID>", pwd, "<enter your domain>");
Process.EnterDebugMode();
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